An improved tropospheric nitrogen dioxide (NO2) retrieval algorithm from the Global Ozone Monitoring Experiment-2 (GOME-2) instrument based on air mas…An improved tropospheric nitrogen dioxide (NO2) retrieval algorithm from the Global Ozone Monitoring Experiment-2 (GOME-2) instrument based on air mass factor (AMF) calculations performed with more realistic model parameters is presented. The viewing angle dependency of surface albedo is taken into account by improving the GOME-2 Lambertian-equivalent reflectivity (LER) climatology with a directionally dependent LER (DLER) dataset over land and an ocean surface albedo parameterisation over water. A priori NO2 profiles with higher spatial and temporal resolutions are obtained from the IFS (CB05BASCOE) chemistry transport model based on recent emission inventories. A more realistic cloud treatment is provided by a clouds-as-layers (CAL) approach, which treats the clouds as uniform layers of water droplets, instead of the current clouds-as-reflecting-boundaries (CRB) model, which assumes that the clouds are Lambertian reflectors. On average, improvements in the AMF calculation affect the tropospheric NO2 columns by ±15 % in winter and ±5 % in summer over largely polluted regions. In addition, the impact of aerosols on our tropospheric NO2 retrieval is investigated by comparing the concurrent retrievals based on ground-based aerosol measurements (explicit aerosol correction) and the aerosol-induced cloud parameters (implicit aerosol correction). Compared with the implicit aerosol correction utilising the CRB cloud parameters, the use of the CAL approach reduces the AMF errors by more than 10 %. Finally, to evaluate the improved GOME-2 tropospheric NO2 columns, a validation is performed using ground-based multi-axis differential optical absorption spectroscopy (MAXDOAS) measurements at different BIRA-IASB stations. At the suburban Xianghe station, the improved tropospheric NO2 dataset shows better agreement with coincident ground-based measurements with a correlation coefficient of 0.94.more
Remote-sensing records over the last 40 years have revealed large year-to-year global and regional variability in Antarctic sea ice extent. Sea ice ar…Remote-sensing records over the last 40 years have revealed large year-to-year global and regional variability in Antarctic sea ice extent. Sea ice area and extent are useful climatic indicators of large-scale variability, but they do not allow the quantification of regions of distinct variability in sea ice concentration (SIC). This is particularly relevant in the marginal ice zone (MIZ), which is a transitional region between the open ocean and pack ice, where the exchanges between ocean, sea ice and atmosphere are more intense. The MIZ is circumpolar and broader in the Antarctic than in the Arctic. Its extent is inferred from satellite-derived SIC using the 15 %-80 % range, assumed to be indicative of open drift or partly closed sea ice conditions typical of the ice edge. This proxy has been proven effective in the Arctic, but it is deemed less reliable in the Southern Ocean, where sea ice type is unrelated to the concentration value, since wave penetration and free-drift conditions have been reported with 100 % cover. The aim of this paper is to propose an alternative indicator for detecting MIZ conditions in Antarctic sea ice, which can be used to quantify variability at the climatological scale on the ice-covered Southern Ocean over the seasons, as well as to derive maps of probability of encountering a certain degree of variability in the expected monthly SIC value. The proposed indicator is based on statistical properties of the SIC; it has been tested on the available climate data records to derive maps of the MIZ distribution over the year and compared with the threshold-based MIZ definition. The results present a revised view of the circumpolar MIZ variability and seasonal cycle, with a rapid increase in the extent and saturation in winter, as opposed to the steady increase from summer to spring reported in the literature. It also reconciles the discordant MIZ extent estimates using the SIC threshold from different algorithms. This indicator complements the use of the MIZ extent and fraction, allowing the derivation of the climatological probability of exceeding a certain threshold of SIC variability, which can be used for planning observational networks and navigation routes, as well as for detecting changes in the variability when using climatological baselines for different periods.more
Arctic sea ice motion information provides an important scientific basis for revealing the changing mechanism of Arctic sea ice and assessing the navi…Arctic sea ice motion information provides an important scientific basis for revealing the changing mechanism of Arctic sea ice and assessing the navigational safety of Arctic waterways. For now, many satellite derived Arctic sea ice motion products have been released but few studies have conducted comparisons of these products. In this study, eleven satellite sea ice motion products from the Ocean and Sea Ice Satellite Application Facility (OSI SAF), the National Snow and Ice Data Center (NSIDC), and the French Research Institute for the Exploitation of the Seas (Ifremer) were systematically evaluated and compared based on buoys from the International Arctic Buoy Program (IABP) and the Multidisciplinary drifting Observatory for the Study of Arctic Climate (MOSAiC) over 2018–2020. The results show that the mean absolute errors (MAEs) of ice speed for these products are 1.15–2.26 km/d and the MAEs of ice motion angle are 14.93–23.19°. Among all products, Ifremer_AMSR2 achieves the best accuracy in terms of speed error, NSIDC_Pathfinder shows the lowest angle error and OSI-405-c_Merged performs best in sea-ice drift trajectory reconstruction. Moreover, season, region, data source, ice drift tracking algorithm, and time interval all influence the accuracy of these products: (1) The sea ice motion bias in the freezing season (1.04–1.96 km/d and 11.93–22.41°) is smaller than that in the melting season (1.13–3.90 km/d and 14.41–27.41°) for most of the products. (2) Most products perform worst in East Greenland, where ice movements are fast and complex. (3) The accuracies of the products derived from AMSR-2 remotely sensed data are better than those from other data sources. (4) The continuous maximum cross-correlation (CMCC) algorithm outperforms the maximum cross-correlation (MCC) algorithm in sea ice drift retrieval. (5) The MAEs of sea ice motion with longer time interval are relatively smaller. Overall, the results indicate that the eleven remote sensing Arctic sea ice drift products are of practical use for data assimilation and model validation if uncertainties are appropriately considered. Furthermore, this study provides some improvement directions for sea ice drift retrieval from satellite data.more
A new generation of cloud radars, with the ability to make observations close to the surface, presents the possibility of observing fog properties wit…A new generation of cloud radars, with the ability to make observations close to the surface, presents the possibility of observing fog properties with better insight than was previously possible. The use of these instruments as part of an operational observation network could improve the prediction of fog events, something which is still a problem for even high-resolution numerical weather prediction models. However, the retrieval of liquid water content (LWC) profiles from radar reflectivity alone is an under-determined problem, something which ground-based microwave radiometer observations can help to constrain. In fact, microwave radiometers are not only sensitive to temperature and humidity profiles but are also known to be instruments of reference for the liquid water path. By providing the thermodynamic state of the atmosphere, to which the formation and evolution of fog events are highly sensitive, in addition to accurate liquid water path, which can be used to constrain the LWC retrieval from the cloud radar alone, combining microwave radiometers with cloud radars seems a natural next step to better understand and forecast fog events. To that end, a newly developed one-dimensional variational (1D-Var) algorithm designed for the retrieval of temperature, specific humidity and liquid water content profiles with both cloud radar and microwave radiometer (MWR) observations is presented in this study. The algorithm was developed to evaluate the capability of cloud radar and MWR to provide accurate LWC profiles in addition to temperature and humidity in view of assimilating the retrieved profiles into a 3D- and 4D-Var operational assimilation system. The algorithm is firstly tested on a synthetic dataset, which allows the evaluation of the developed algorithm in idealised conditions. This dataset was constructed by perturbing a high-resolution forecast dataset of fog and low-cloud cases by its expected errors. The algorithm is then tested with real data from the recent field campaign SOFOG-3D, carried out with the use of LWC measurements made from a tethered balloon platform. As expected, results from the synthetic dataset study were found to contain lower errors than those found from the retrievals on the dataset of real observations. It was found that LWC can be retrieved in idealised conditions with an uncertainty of less than 0.04 g m(-3). With real data, as expected, retrievals with a good correlation (0.7) to in situ measurements were found but with a higher uncertainty than the synthetic dataset of around 0.06 g m(-3) (41 %). This was reduced to 0.05 g m(-3) (35 %) when an accurate droplet number concentration could be prescribed to the algorithm. A sensitivity study was conducted to discuss the impact of different settings used in the 1D-Var algorithm and the forward operator. Additionally, retrievals of LWC from a real fog event observed during the SOFOG-3D field campaign were found to significantly improve the operational background profiles of the AROME (Application of Research to Operations at MEsoscale) model, showing encouraging results for future improvement of the AROME model initial state during fog conditions.more
Abstract The Coordinating Earth Observation Data Validation for Reanalysis for Climate Services project (CORE-CLIMAX) aimed to substantiate how Copern…Abstract The Coordinating Earth Observation Data Validation for Reanalysis for Climate Services project (CORE-CLIMAX) aimed to substantiate how Copernicus observations and products can contribute to climate change analyses. CORE-CLIMAX assessed the European capability to provide climate data records (CDRs) of essential climate variables (ECVs), prepared a structured process to derive CDRs, developed a harmonized approach for validating essential climate variable CDRs, identified the integration of CDRs into the reanalysis chain, and formulated a process to compare the results of different reanalysis techniques. With respect to the Copernicus Climate Change Service (C3S), the systematic application and further development of the CORE-CLIMAX system maturity matrix (SMM) and the spinoff application performance metric (APM) were strongly endorsed to be involved in future implementations of C3S. We concluded that many of the current CDRs are not yet sufficiently mature to be used in reanalysis or applied in climate studies. Thus, the production of consistent high-resolution data records remains a challenge that needs more research urgently. Extending ECVs to close climate cycle budgets (e.g., essential water variables) is a next step linking CDRs to sectoral applications.more
To date, there is no long-term, stable, and uncertainty-quantified dataset of upper tropospheric humidity (UTH) that can be used for climate research.…To date, there is no long-term, stable, and uncertainty-quantified dataset of upper tropospheric humidity (UTH) that can be used for climate research. As intermediate step towards the overall goal of constructing such a climate data record (CDR) of UTH, we produced a new fundamental climate data record (FCDR) on the level of brightness temperature for microwave humidity sounders that will serve as basis for the CDR of UTH. Based on metrological principles, we constructed and implemented the measurement equation and the uncertainty propagation in the processing chain for the microwave humidity sounders. We reprocessed the level 1b data to obtain newly calibrated uncertainty quantified level 1c data in brightness temperature. Three aspects set apart this FCDR from previous attempts: (1) the data come in a ready-to-use NetCDF format; (2) the dataset provides extensive uncertainty information taking into account the different correlation behaviour of the underlying errors; and (3) inter-satellite biases have been understood and reduced by an improved calibration. Providing a detailed uncertainty budget on these data, this new FCDR provides valuable information for a climate scientist and also for the construction of the CDR.more
Abstract Insufficient understanding of complex Arctic cloud properties introduced large errors in estimating radiant energy balance parameters at the …Abstract Insufficient understanding of complex Arctic cloud properties introduced large errors in estimating radiant energy balance parameters at the regional and global scales. Comprehensive and reliable cloud information is necessary for improving the accuracy of flux inversion. This study evaluated daytime cloud fraction (CF) uncertainties from 16 available satellite products and estimated the spatiotemporal distributions of Arctic daytime CF during 2000–19. Our results show that the differences among multiple products had significant temporal and spatial heterogeneities. Temporally, the maximum and minimum interproduct discrepancies occurred in April and the summer months, respectively. Spatially, the largest uncertainties were seen over Greenland. Substantial inconsistency also occurred on the central and Pacific sides of the Arctic Ocean. The active satellite product tended to capture more clouds in these two regions. We found that the inconsistencies caused by sensor differences were smaller than those caused by algorithm differences; that is, for MODIS based CF products, the inconsistencies caused by different sensors and different algorithms are ±2% and ±5%, while for AVHRR-based products, these inconsistencies are ±6% and ±15%, respectively. The annual average daytime CF in sunlit months was 70.9% ± 2.93% and increased over the Arctic during study periods. These upward trends might cool the Arctic by approximately 0.05–0.5 W m−2 decade−1. In terms of the spatiotemporal distributions, the CF over the ocean is higher than that over the land, and the former increased significantly while the latter decreased; the CF trends of most products are positive in June and July but are opposite in other months. From this study, the findings based on multiple products would be more robust than that based on a single or few datasets. Significance Statement This study aimed to comprehensively understand and obtain more robust general characteristics of the temporal and spatial distributions of Arctic daytime cloud fraction by comparing and analyzing the consistencies and discrepancies of multisource satellite products. It is important because the cloud fraction is a nonnegligible modulator of Earth’s energy budget and climate change. Although the Arctic is the most climate-sensitive region, existing studies lack a comprehensive assessment of the cloud fraction over the entire Arctic. We analyzed 16 different cloud products and found that although the inconsistencies were inevitable, most products showed similar spatiotemporal distribution and trend distribution of daytime CF. This study provided a new idea for Arctic CF research under the existing conditions.more